The diffusion-limited reaction A + A-+ 0 in the steady state: influence of correlations in the source

نویسنده

  • E. Clement
چکیده

We study theoretically the kinetics of the diffusion-limited reaction A+A-+O in the steady state. We consider the effect of an external source which adds correlated pairs of particles. We show that in dimensions below 2 and in the low-density limit spatial self-organization of reactants occurs and is controlled by the correlation in the source term. At higher densities there is a crossover to a regime similar to the random landing case, exhibiting a non-classical order of reaction.

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تاریخ انتشار 2001